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Spin tunneling in magnetic molecules

Posted on:2006-04-09Degree:Ph.DType:Thesis
University:Northwestern UniversityCandidate:Kececioglu, ErsinFull Text:PDF
GTID:2450390008474909Subject:Physics
Abstract/Summary:
In this thesis, we will focus on spin tunneling in a family of systems called magnetic molecules such as Fe8 and Mn12. This is comparatively new, in relation to other tunneling problems. Many issues are not completely solved and/or understood yet. The magnetic molecule Fe 8 has been observed to have a rich pattern of degeneracies in its magnetic spectrum. We focus on these degeneracies from several points of view.; We start with the simplest anisotropy Hamiltonian to describe the Fe 8 molecule and extend our discussion to include higher order anisotropy terms. We give analytical expressions as much as we can, for the degeneracies in the semi-classical limit in both cases. We reintroduce jump instantons to the instanton formalism.; Finally, we discuss the effect of the environment on the molecule. Our results, for all different models and techniques, agree well with both experimental and numerical results.
Keywords/Search Tags:Molecule, Magnetic, Tunneling
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